2011-12-14
Attosecond control of dissociative ionization of O2 molecules
Publication
Publication
Phys. Rev. A , Volume 84 - Issue 6, Article number: 63412 p. 1- 4
We demonstrate that dissociative ionization of O2 can be controlled by the relative delay between an attosecond pulse train (APT) and a copropagating infrared (IR) field. Our experiments reveal a dependence of both the branching ratios between a range of electronic states and the fragment angular distributions on the extreme ultraviolet (XUV) to IR time delay. The observations go beyond adiabatic propagation of dissociative wave packets on IR-induced quasistatic potential energy curves and are understood in terms of an IR-induced coupling between electronic states in the molecular ion.
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APS | |
doi.org/10.1103/PhysRevA.84.063412 | |
Phys. Rev. A | |
Siu, W., Kelkensberg, F., Gademann, G., Rouzée, A., Johnsson, P., Dowek, D., … Vrakking, M. J. J. (2011). Attosecond control of dissociative ionization of O2 molecules. Phys. Rev. A, 84(6, Article number: 63412), 1–4. doi:10.1103/PhysRevA.84.063412 |